Why not just remove the overload spring pack and see what difference it makes? It won't cost a dime and you will be afforded the chance to revive the effects for yourself, not through some third person opinion.
I removed my overloads about a year ago, I like the trucks highway ride much better. If you tow very heavy loads, you might want to consider air bags, they can give you the support you need with out the rough ride. But that is something you can determine latter. I only know of the T-Rex (Yell I know, but i like that name better) mini packs. They do have tapered leafs, and are a direct replacement for the Overload springs, nothing to do with the main springs. If you want to experiment with the main spring pack, then remove one of the leafs and try it. Another option is to contact National Spring, they will custom make you a rear set of leaf springs for around 300 bucks a set.
For shocks I am not all that happy with Rancho's, I have used them in the past and have had problems with them leaking. The Bilstien OEM 5100 series are nice shocks, but they are also firmer shocks. This might be counterproductive to want you are trying to achieve, don't know? Their are many companies out now with higher end shocks that can be rebuilt and re-valved. This might be worth considering, depends on your budget and commitment to the smooth ride . I have made great strides toward the smooth highway ride, eliminating the rear overloads was the best move so far. That allowed the rear suspension to travel much further without bashing into the overload spring stops, the result a much smoother ride. When not loaded, I keep just enough air in the rear bags to take the weight of the truck off the rear springs, this really helps smooth out the small bumps and expansion cracks on the highway, the bags take the shock and not the truck.
I have decided to take my trucks suspension to the next level, I liked the T-Rex suspension Ideal so I went with the Fox shocks all around and dual Fox shocks on each side up front. It's kind of an experiment, I wanted to see the benefits of dual shocks up front. I will not get them mounted up till spring, I have them hanging up in the garage where I see them everyday teasing me, but I'll wait till spring. Many of the front end parts I ordered have not come in yet, some are on back order for 2-3 week which will put us into the cold winter weather, not working outside weather.
There is no set way to make your truck ride better, you can do a number of things that will help, the decision is yours to make. I just wanted to post and tell you what I have done, and how it effected the ride. I am also considering a new set of rear springs from Nation Spring, I like the ideal of replacing the stock ones. Let us know what you decided to do and how it effected the ride quality, good luck.